Quantum Matter

Recently, a new family of correlated honeycomb materials with strong spin-orbit coupling have been promising candidates to realize the Kitaev spin liquid. In particular, a half-integer quantized thermal Hall conductivity was reported in alpha-RuCl3 under the magnetic field. Using a generic nearest neighbour spin model with bond-dependent interactions, I will present numerical evidence of an extended regime of quantum spin liquids. I will also discuss how to achieve a chiral spin liquid near ferromagnetic Kitaev interaction in the presence of the magnetic field leading to the quantized thermal Hall conductivity.

Kitaev materials — spin-orbit assisted Mott insulators, in which local, spin-orbit entangled j=1/2 moments form that are subject to strong bond-directional interactions — have attracted broad interest for their potential to realize spin liquids. Experimentally, a number of 4d and 5d systems have been widely studied including the honeycomb materials Na2IrO3, α-Li2IrO3, and RuCl3 as candidate spin liquid compounds — however, all of these materials magnetically order at sufficiently low temperatures. In this talk, I will discuss the physics of Kitaev materials that plays out when applying magnetic fields. Experiments on RuCl3 indicate the formation of a chiral spin liquid that gives rise to an observed quantized thermal Hall effect. Conceptually, this asks for a deeper understanding of the physics of the Kitaev model in tilted magnetic fields. I will report on our recent numerical studies that give strong evidence for a Higgs transition from the well known Z2 topological spin liquid to a gapless U(1) spin liquid with a spinon Fermi surface and put this into perspective of experimental studies.

We study the eigenstate properties of a nonintegrable spin chain that was recently realized experimentally in a Rydberg-atom quantum simulator. In the experiment, long-lived coherent many-body oscillations were observed only when the system was initialized in a particular product state. This pronounced coherence has been attributed to the presence of special "scarred" eigenstates with nearly equally-spaced energies and putative nonergodic properties despite their finite energy density. In this paper we uncover a surprising connection between these scarred eigenstates and low-lying quasiparticle excitations of the spin chain. In particular, we show that these eigenstates can be accurately captured by a set of variational states containing a macroscopic number of magnons with momentum π. This leads to an interpretation of the scarred eigenstates as finite-energy-density condensates of weakly interacting π-magnons. One natural consequence of this interpretation is that the scarred eigenstates possess long-range order in both space and time, providing a rare example of the spontaneous breaking of continuous time-translation symmetry. We verify numerically the presence of this space-time crystalline order and explain how it is consistent with established no-go theorems precluding its existence in ground states and at thermal equilibrium.

We study the possibility of a deconfined quantum phase transition in a realistic model of a two dimensional Shastry-Sutherland quantum magnet, using both numerical and field theoretic techniques. We argue that the quantum phase transition between a two fold degenerate plaquette valence bond  solid (pVBS) order and N\'eel ordered phase may be described by a deconfined quantum critical point (DQCP) with emergent O(4) symmetry. Further, using the infinite density matrix renormalization group (iDMRG) numerical technique, we verify the emergence of an intermediate pVBS order, between the dimer and Neel ordered phases. By analyzing the correlation length spectrum, we provide evidence for deconfinement and emergent O(4) symmetry at the phases transistion between the pVBS and N\'eel orders. Such a phase transition has been reported in the recent pressure tuned experiments in the Shastry-Sutherland lattice material  SrCu2(BO3)2. The non-symmorphic lattice structure of the Shastry-Sutherland compound leads to extinction points in the scattering, where we predict sharp signatures of a DQCP in both the phonon and magnon spectra associated with the spinon continuua. Our results can guide future experimental studies of DQCP in quantum magnets.

The construction of soluble lattice toy models is an important theoretical approach in the study of strongly interacting topological phases of matter. On the other hand, the primary experimental probe to such systems is via electromagnetic response. Somewhat unsatisfactorily, the current systematic construction of the lattice toy models focuses on braiding statistics and does not admit coupling to an electromagnetic background. Thus there is a mismatch between our theoretical approach and experimental probe. In this talk I introduce how to systematically incorporate electromagnetic response into the soluble lattice toy models, for a large class of abelian topological phases. [Reference: 1902.06756] 

Experiments with ultracold fermionic gases are thriving and continue to provide us with valuable insights into fundamental aspects of physics. A special system of interest is the so-called unitary Fermi gas (UFG) situated right in the "middle" of the crossover between Bardeen-Cooper-Schrieffer superfluidity and Bose-Einstein condensation. However, the theoretical treatment of these gases is highly challenging due to the absence of a small expansion parameter as well as the appearance of the infamous sign problem in the presence of, e.g., finite spin polarizations. In this talk, I will discuss the concept of stochastic quantization and motivate the complex Langevin (CL) method for non-relativistic fermions as an alternative to conventional Monte Carlo approaches. In particular, I will show how the CL approach can be employed to study the spin-polarized UFG. In the unpolarized limit, our results for the EOS are in excellent agreement with the existing state-of-the-art results from other ab-initio approaches as well as with experimental data. For the polarized case, our results for the EOS and other thermodynamic quantities represent experimentally testable predictions, already providing us with some insight into the underlying phase diagram.

In crystals, quantum electrons can be spatially distributed in a way that the bulk solid supports macroscopic electric multipole moments, which are deeply 

related with emergence of topology insulators in condensed matter systems. However, unlike the classical electric multipoles in open space, 

defining electric multipoles in crystals is a non-trivial task. So far, only the dipolar moment, namely polarization, has been successfully defined and served as a classic example of topological insulators. 

In this talk, we propose the general definition, i.e., many-body invariants, for electric multipoles in crystals, which are related with recently-discovererd higher-order topological insulators. 

Our invariants are designed to measure the distribution of electron charge in unit cells and thus can detect multipole moments purely from the bulk ground state wavefunctions. 

We provide analytic as well as numerical proofs for our invariants. Application of our invariants to spin systems as well as various other aspects of the many-body invariants will be briefly discussed.

This seminar will focus on two cases where the interplay of topology and interactions allows for phases that go beyond simple quasi-particle descriptions. Both models are amenable to sign free auxiliary field quantum Monte Carlo simulations.

First, we design a two-dimensional model consisting of four Dirac-fermion layers on the square lattice. The interaction is given by a four-fermion term where each fermion is from a different layer. In the uncorrelated case, the topology is determined by a Z-valued winding number and previous studies, often using the bulk-boundary correspondence and dimensional reduction arguments, predict the reduction to a Z4 classification in the presence of correlations. An adiabatic path between formerly distinct phases has to visit a strongly interacting state that cannot be described on a mean-field level. We study the phase diagram of the full bulk system and find a symmetry broken state separating topological distinct phases. An attempt to frustrate the ordered state introduces a first order phase transition [Fig. 1 (left)].

Second, we consider Dirac electrons on the honeycomb lattice Kondo coupled to spin-1/2 degrees of freedom on the kagome lattice. The interactions between the spins are chosen along the lines of the Balents-Fisher-Girvin model that is known to host a Z2 spin liquid and a fer- romagnetic phase. While in the ferromagnetic phase the Dirac electrons acquire a gap, they remain massless in the Z2 spin liquid phase due to the breakdown of Kondo screening. Since our model has an odd number of spins per unit cell, this phase is a non-Fermi liquid, also called fractionalized Fermi liquid, that violates the conventional Luttinger theorem, which relates the Fermi volume to the particle density in a Fermi liquid. We probe the Kondo breakdown in this non-Fermi liquid phase via conventional observables such as the spectral function, and also by studying the mutual information between the electrons and the spins [Fig. 1 (right)].

Figure 1: Schematic sketch of the phase diagram discussed during the beginning of the seminar (left). Numerical Results consistent with a FL* to magnetic insulator transition as subject of the second half (right).

In our previous work (Phys. Rev. Lett. 121, 046401 (2018)), we found a quantum spin liquid phase with spinon Fermi surface in the two dimensional spin-1/2 Heisenberg model with four-spin ring exchange on a triangular lattice. In this work we dope the spinon Fermi surface phase by studying the t-J model with four-spin ring exchange. We perform density matrix renormalization group calculations on four-leg cylinders of a triangular lattice and find that the dominant pair correlation function is that of a pair density wave, i.e. it is oscillatory while decaying with distance with a power law. The doping dependence of the period is studied. This is the first example where pair density wave is the dominant pairing in a generic strongly interacting system where the pair density wave cannot be explained as a composite order and no special symmetry is required. Reference: 1. arXiv:1803.00999 [cond-mat.str-el] (Phys. Rev. Lett. 121, 046401 (2018)) 2. arXiv:1811.06538 [cond-mat.str-el]

Systems of strongly interacting particles can give rise to topological phases beyond non-interacting limit.  Although unique features of strongly interacting topological phases, such as fractionalization of quantum degrees of freedom, have important applications in quantum information processing, these topological phases are still far from experimental realizations. In this talk, by presenting constructions of two strongly interacting topological phases, I will argue the key mechanism of their realizations is to add interactions near topological phase transitions.  I will first introduce a model of interacting Majorana fermions that describes a superconducting phase with Fibonacci topological order. Then I will show that a correlated fluid of electrons and holes, dubbed fractional excitonic insulator phase, can exhibit a fractional quantum Hall effect at zero magnetic field. I will present physical evidence and conjecture that this phase can be realized in a higher angular momentum excitonic paired system in the presence of interactions.   

Finding a quantum phase transition between two even well-studied phases of matter can be a hard problem. Free probability theory suggests a new method which can give an answer if the Hamiltonians of two phases satisfy certain conditions. In the latter case, the spectral gap behavior can be calculated without solving the full Hamiltonian but using probabilistic estimation instead. As an example, I will consider generic artificial topological systems created by a periodic drive, including Floquet Majorana modes, and show how FPT can be used to predict and characterize disorder-driven phase transitions.

See also: Phys. Rev. Lett. 121, 126803

Interacting electrons in high magnetic fields exhibit rich physical phenomena including the gapped fractional quantum Hall effects and the gapless states. The composite Fermi liquids (CFLs) are gapless states that can occur at even denominator Landau level fillings. Due to the celebrated work of Halperin, Lee and Read (94), the CFLs were understood as Fermi liquids of composite fermions, which are bound states of electron and electromagnetic flux quanta. However, at 1/2 filling, it is not obvious why the HLR description is consistent with the particle hole symmetry. Motivated by this, recently Son (15) proposed an alternative description for CFLs at 1/2, according to which the composite fermions are instead emergent Dirac fermions. Importantly, Son’s theory predicts a Pi Berry curvature singularity at the composite Fermi sea center. In the first part of this talk [2,3], I will present our numerical work about detecting this Z2 Berry phase at 1/2 filling. In the second part [1], I will present how and why Dirac fermions can emerge at all the other filling fractions (1/2m and 1-1/2m when m is integer) even without the particle hole symmetry.

[1] arXiv 1808.07529. JW.

[2] arXiv 1711.07864. Geraedts, JW, Rezayi, Haldane.

[3] arXiv 1710.09729. JW, Geraedts, Rezayi, Haldane.