Condensed Matter

Kitaev materials — spin-orbit assisted Mott insulators, in which local, spin-orbit entangled j=1/2 moments form that are subject to strong bond-directional interactions — have attracted broad interest for their potential to realize spin liquids. Experimentally, a number of 4d and 5d systems have been widely studied including the honeycomb materials Na2IrO3, α-Li2IrO3, and RuCl3 as candidate spin liquid compounds — however, all of these materials magnetically order at sufficiently low temperatures. In this talk, I will discuss the physics of Kitaev materials that plays out when applying magnetic fields. Experiments on RuCl3 indicate the formation of a chiral spin liquid that gives rise to an observed quantized thermal Hall effect. Conceptually, this asks for a deeper understanding of the physics of the Kitaev model in tilted magnetic fields. I will report on our recent numerical studies that give strong evidence for a Higgs transition from the well known Z2 topological spin liquid to a gapless U(1) spin liquid with a spinon Fermi surface and put this into perspective of experimental studies.

We study the eigenstate properties of a nonintegrable spin chain that was recently realized experimentally in a Rydberg-atom quantum simulator. In the experiment, long-lived coherent many-body oscillations were observed only when the system was initialized in a particular product state. This pronounced coherence has been attributed to the presence of special "scarred" eigenstates with nearly equally-spaced energies and putative nonergodic properties despite their finite energy density. In this paper we uncover a surprising connection between these scarred eigenstates and low-lying quasiparticle excitations of the spin chain. In particular, we show that these eigenstates can be accurately captured by a set of variational states containing a macroscopic number of magnons with momentum π. This leads to an interpretation of the scarred eigenstates as finite-energy-density condensates of weakly interacting π-magnons. One natural consequence of this interpretation is that the scarred eigenstates possess long-range order in both space and time, providing a rare example of the spontaneous breaking of continuous time-translation symmetry. We verify numerically the presence of this space-time crystalline order and explain how it is consistent with established no-go theorems precluding its existence in ground states and at thermal equilibrium.